It depends on what you need. If you only want 25 to 50Hz to help the pair of 4520 scoops, then I would go with a TCB. If you want stand alone bass bins that cover 30 to 200 Hz, the sure, the 4641 would be better. BTW I can lend you my 1800 Gti to test against your 2241. They share the same basket and motor. I suspect the 1800Gti to be less musical but more bass heavy.
GTI 1800
Mechanical parameters
Fs = 30hz
Qms = 6,77
Vas = 362,46 Liters
Cms = 0,158 mm/N
Mms = 178,141 grams
Rms = 4,96 kg/sec
Xmax = 7,62 mm
Sd = 1271 sq.cm
Dia = 40,2 cm
Electrical parameters
Qes = 0,456
Re = 2,5 ohms
Le = 1 mh
Z = 4 ohms
BL = 13,6 N/A
Pe = 600 Watts
Kombination parameters
Qts = 0,43
n* = 2,07%
Sens = 96,3 (1 Watt)